ArticleScience advances2026
Real-time direct detection of Criegee intermediates from ozonolysis of alkenes in an atmospheric simulation chamber.
Article in Science advances, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Authors and funding
5 authors.
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Abstract
Ozonolysis reactions are key oxidation mechanisms for unsaturated volatile organic compounds in the atmosphere, generating Criegee intermediates (CIs) that drive subsequent chemistry. Photolytic laboratory sources of certain CIs have demonstrated unexpectedly high CI reactivity but bypass the complex dynamics that occur in the atmosphere during ozonolysis, which affect yields and reactivity. Here, we report direct measurements of absolute concentrations of the CIs formaldehyde oxide (CH
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