ArticleACS applied materials & interfaces2026
Block Copolymer-Enabled Low-Temperature Structural Battery Electrolytes Produced Using Polymerization-Induced Phase Separation.
Article in ACS applied materials & interfaces, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Structural battery electrolytes (SBEs) require both high ionic conductivity and high mechanical strength and stiffness. However, SBEs produced using the one-pot polymerization-induced phase separation (PIPS) synthesis method suffer from high tortuosity which decreases the effective ionic conductivity. Additionally, conventional liquid electrolytes demonstrate poor performance in low temperatures and are unsuitable for applications in cold climates. Here, we report SBEs generated using PIPS in the presence of an amphiphilic block copolymer (BCP), which modifies the solid-liquid interface that forms during polymerization, resulting in lower tortuosity and improved ionic conductivity. Using a low-temperature liquid electrolyte, the effect of BCP and resin content on the ionic conductivity and mechanical properties is examined. Only 1 wt % of BCP additive is needed to improve the ionic conductivities even at low temperature (2.34 × 10
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