ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026
Interfacially Reinforced Crosslinked Binder with Structural Integrity for Stable Micro-Sized Silicon Anodes in All-solid-state Batteries.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
All-solid-state batteries (ASSBs) have attracted considerable attention as next-generation energy storage systems owing to their high energy density and safety. However, their performance is critically limited by insufficient solid-solid interfacial contact and severe chemomechanical degradation, particularly for micro-sized silicon (µSi) anodes that undergo large volume changes during cycling. In this study, we report an interfacially reinforced crosslinked binder (IRCB) designed to stabilize µSi anodes in ASSBs by simultaneously addressing mechanical integrity and interfacial stability. The IRCB is synthesized via a facile crosslinking reaction between 1,4-butanediol diglycidyl ether and ethylenediamine, forming a robust 3D polymer network. This crosslinked structure enhances mechanical constraint, maintains interparticle contact, and provides ether-rich domains that facilitate Li
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