ArticleMaterials horizons2026
Thermal-driven H-bond reconfiguration for bioinspired high-strength anisotropic supramolecular hydrogels.
Article in Materials horizons, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Natural anisotropic tissues, such as tendons and cartilages, achieve remarkable mechanical properties and various biofunctions through oriented hierarchical structures. Inspired from organisms, we develop a synergistic molecular and structural engineering technique based on the thermodynamically reversible reconfiguration of hydrogen bonds to achieve high-performance anisotropic supramolecular hydrogels by quenching pre-stretched polymer networks. Multiple inherent hydrogen bonds gradually dissociate under high-temperature processing to allow the good alignment of the polymer chains by uniaxial pre-stretching. The oriented polymer chains are then fixed on-site by rapid quenching-mediated hydrogen bond reconstruction at low temperatures (
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