ArticleACS omega2026
Interfacial Curing Kinetics and Compatibilization Behavior of NR/HNBR/ENR Blends: Morphology, Viscoelasticity, and Network Structure.
Article in ACS omega, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. An erratum has been issued. Not yet cited in PubMed.
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Corrections and comments
- Erratum issued
Authors and funding
8 authors.
Funding
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Abstract
The development of high-performance elastomers that reconcile the conflicting requirements of cryogenic flexibility, oil resistance, and dynamic durability remains a formidable challenge. Here, we investigate interfacial compatibilization and vulcanization kinetics in natural rubber/hydrogenated nitrile butadiene rubber (NR/HNBR) blends using epoxidized natural rubber (ENR) as a compatibilizer. We demonstrate that the vulcanization kinetics and properties of these immiscible constituents are governed not only by thermodynamic compatibility but, more critically, by the kinetically driven migration of curatives (sulfur and accelerators) across the phase boundaries. Atomic force microscopy (AFM) and dynamic mechanical analysis (DMA) show that ENR refines the phase morphology and improves interfacial compatibility. Upon incorporating 8 phr ENR into an NR/HNBR (80/20) blend, the interfacial roughness (
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