ReviewACS applied materials & interfaces2026
Quantum Rate Dynamics for Coherent Electron Transport at Material/Electrolyte Interfaces.
Review in ACS applied materials & interfaces, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Nanoscale electronics and electrochemistry are both based on the fundamental principles of electron motion at the material/electrolyte interfaces. Despite this common ground, these fields use distinct conceptual frameworks: physicists favor coherent electron transport, while chemists rely on kinetic electron transfer. In this work, we present the fundamental quantum-mechanical principles that unify these approaches, linking quantum transport to the electron-transfer rate constant in an electrolyte environment. We show that─even at room temperature─electron motion between quantum states, which appears as a slow kinetic rate, is in fact driven by underlying coherent quantum dynamics, modulated by the electrolyte's damping. This coherent transport determines the kinetics of redox switches, controls biological processes such as Geobacter respiration, enables the development of
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