ArticleNature communications2026
Superior energy storage performance via engineering crossover region with competing orders in high-entropy multilayer capacitors.
Tao Deng, Jiyang Xie, Zhen Liu, Liqiang He, Zhichao Hong, Haonan Peng, Dong Wang, Cosme Milesi-Brault, Teng Lu, Yonghong Chen and 6 more
Abstract read
In one paragraphArticle in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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16 authors.
Tao Deng *Key Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, China.
Jiyang Xie *Yunnan Key Laboratory of Electromagnetic Materials and Devices, National Center for International Research on Photoelectric and Energy Materials, School of Materials and Energy, Yunnan University, Kunming, China.ORCID http://orcid.org/0000-0003-0419-9830 Zhen LiuKey Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, China. zhenliu@mail.sic.ac.cn.ORCID http://orcid.org/0000-0003-4895-0948 Zhichao HongTorch Electron Technology Co., LTD, Quanzhou, Fujian, China.
Haonan PengKey Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, China.
Dong WangFrontier Institute of Science and Technology and State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, China. wang_dong1223@mail.xjtu.edu.cn.ORCID http://orcid.org/0000-0001-6009-166X Teng LuResearch School of Chemistry, The Australian National University, Canberra, ACT, Australia.
Yonghong ChenTorch Electron Technology Co., LTD, Quanzhou, Fujian, China.
Zhisheng LinTorch Electron Technology Co., LTD, Quanzhou, Fujian, China.
Wanbiao HuYunnan Key Laboratory of Electromagnetic Materials and Devices, National Center for International Research on Photoelectric and Energy Materials, School of Materials and Energy, Yunnan University, Kunming, China.ORCID http://orcid.org/0000-0003-0180-9648 Genshui WangKey Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, China. genshuiwang@mail.sic.ac.cn.ORCID http://orcid.org/0000-0002-5077-6574 Junhao ChuState Key Laboratory of Infrared Physics, Shanghai Institute of Technical Physics, Chinese Academy of Sciences, Shanghai, China.
Funding
National Natural Science Foundation of China (National Science Foundation of China) 12204503National Natural Science Foundation of China (National Science Foundation of China) U2002217Natural Science Foundation of Shanghai (Natural Science Foundation of Shanghai Municipality) 23ZR1472400
6 · The paper itselfAbstract
As promising candidates for next-generation energy storage devices in electrical and electronic systems, lead-free multilayer ceramic capacitors face increasingly high performance requirements. To counteract the usual trade-off between energy storage density and efficiency, we here propose a high-entropy design that directly harnesses diverse oxide symmetries to targetedly engineer competing orders and tune the composition into the crossover region between relaxor ferroelectric and superparaelectric states. Atomic-scale structural analysis reveals high-entropy ceramic develops pronounced local polarization fluctuation and dispersed oxygen octahedral rotations, which enhance relaxor behavior and reduce switching barrier. Consequently, superior recoverable energy density of 20.64 J cm
Identifiers
PMID41673390
PMCPMC13004956
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