ArticleAngewandte Chemie (International ed. in English)2026
Proton Tautomerism for Anhydrous Superprotonic Conduction in 1,2,3-Triazolium Dihydrogen Phosphate Crystal.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Proton dynamics within molecular organic solids are crucial for energy-related technologies. Proton conductors for use as solid electrolytes in hydrogen fuel cells have been developed, elucidating the higher proton transport mechanism and establishing design guidelines for higher conduction. Many anhydrous proton conductors for proton transport utilizing molecular motion in solids have been studied; however, low-barrier conduction is challenging. In this study, we addressed proton tautomerism as a new guideline for proton conduction, rather than molecular motion. The key to facilitating low-barrier conduction is proton transport without molecular motion via dynamic interconversion between multiple tautomers. We demonstrated the effectiveness of proton-tautomerism strategy in 1,2,3-triazole dihydrogen phosphate crystal, which exhibited low-barrier, isotropic superprotonic conductivity exceeding 10
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