ArticleACS omega2025
A Hierarchical Enzyme-Mimetic Supramolecular Catalyst Derived from Folic Acid-KOH/Cu Hydrogel: Self-Assembly Study and Mechanism for Enhanced Oxidation of Phenolic Compounds.
Article in ACS omega, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
The rational design of enzyme-mimetic catalysts through supramolecular self-assembly offers a promising avenue for robust, cost-effective, and tunable green catalysis avoiding biological limitations. In this work, we demonstrate the development of a hierarchical supramolecular catalyst derived from folic acid (FA), a natural low-molecular-weight gelator (LMWG), through a two-step process involving pH-triggered self-assembly and copper-(II)-induced hydrogelation. FA was first solubilized in aqueous KOH (pH ≈ 8.5) to form folate ions, which underwent time-dependent self-assembly into fibrillar structures. Upon addition of Cu-(II), these self-assembled structures cross-linked into a stable hydrogel matrix (
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