ArticleNature chemistry2026
Stereoselective total synthesis of skew-tetramantane.
Article in Nature chemistry, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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1 citing paper in PubMed.
- Stereoselective total synthesis of skew-tetramantane.Nature chemistry · 2026Article
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2 authors.
Funding
Abstract
Diamond's elementary chiral constituent-skew-tetramantane-features extreme rigidity, stability and a precisely defined geometry, epitomizing the parent structure of a σ-helicene. While skew-tetramantane is naturally occurring in trace fractions in fossil fuels, efforts over several decades towards its selective synthesis remained unfruitful. With the recent advances in photocatalysis and transition metal catalysis to tame radical and carbene species, we have now devised a targeted total synthesis of skew-tetramantane by means of a stereoselective adamantalogous cage extension. A first cap attachment was effected by a photocatalytic Giese reaction, while remarkable regio-, diastereo- and enantiocontrol were achieved by an intramolecular C(sp
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