ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026
From Solution to Surface: How the Catalytic Environment Modulates Peptide Bond Cleavage by Metal-Oxo Cluster Nanozymes.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Nanozymes that selectively cleave proteins offer a promising alternative to natural proteases due to their superior stability, tunability, and scalability. However, they are either water-soluble, preventing efficient recovery and limiting their practical application, or structurally ill-defined and insoluble, hindering mechanistic understanding and rational catalyst design. To address this, we developed a structurally well-defined dodecanuclear hafnium-based metal-oxo cluster with a tunable solubility that enables direct comparison of homogeneous and heterogeneous catalytic behavior in peptide bond hydrolysis. The soluble cluster, Hf
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