ArticleACS applied engineering materials2025
Boronium Ionic Liquids for High-Voltage Supercapacitors.
Article in ACS applied engineering materials, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Boronium ionic liquids (BILs) are an emergent class of electrolytes with high electrochemical stability afforded by charge delocalization across the cation. BILs are of particular interest for electrochemical energy storage (EES) devices because of their large voltage window. Here, a series of BILs were systematically evaluated as electrolytes in symmetric double-layer capacitors equipped with carbon nanofoam paper (CNFP) architected electrodes. First, the operational voltage window and capacitive properties of supercapacitor cells composed of BILs and CNFP electrodes were evaluated in a two-electrode configuration by using cyclic voltammetry (CV). Then, galvanostatic charge-discharge (GCD) cycling was used to assess the capacitance, energy density, power density, and long-term stability of cells assembled with the BIL electrolyte. Our results show excellent capacitive behavior of the cells assembled with a series of ammonium-, imidazolium-, and pyrrolidinium-based BILs, with nearly rectangular CV curves across a range of scan rates. Specifically, the methylpyrrolidinium-substituted BIL electrolyte ([(1-m-pyrr)-N
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