ArticleACS macro letters2026
Charge Regulation Enables Uptake of Ampholytes to Polyelectrolyte Brushes.
Article in ACS macro letters, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Uptake of proteins and ampholytic solutes into polyelectrolyte brushes underlies some biological processes and also applications in sensing or biomedicine. Especially uptake on the "wrong" side of the isoelectric point (pI) remains puzzling, with charge regulation and solute patchiness proposed as possible mechanisms. Using a hierarchy of approximations, coarse-grained molecular simulations, self-consistent mean-field, and a simple phenomenological model, we investigated the uptake of model ampholytic solutes into polyanionic brushes across varying pH, salt concentrations, p
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