Evidence map›Paper›PMID 41444241›Full record

ArticleNature communications2025

Sustainable polyolefin upcycling using liquid organic hydrogen carrier based hydrogen delivery and hydrocracking.

Taeeun Kwon, Seoyoung Ahn, Taehyup Kim, Jong Hun Kang, Soohwa Jeong, Ki Hyuk Kang, Wangyun Won, Insoo Ro

Abstract read
In one paragraph

Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

0numbers the graph read from it
0cells of the map it votes in
1citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

1 citing paper in PubMed.

  1. Review
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

8 authors.

Taeeun Kwon *Department of Chemical and Biological Engineering, Korea University, Seoul, 02841, Republic of Korea.ORCID http://orcid.org/0009-0007-7661-485X
Seoyoung Ahn *Department of Chemical and Biological Engineering, Korea University, Seoul, 02841, Republic of Korea.
Taehyup KimDepartment of Chemical and Biomolecular Engineering, Seoul National University of Science and Technology, Seoul, 01811, Republic of Korea.ORCID http://orcid.org/0000-0001-8633-1609
Jong Hun KangSchool of Chemical and Biological Engineering and the Institute of Chemical Processes, Seoul National University, Seoul, 08826, Republic of Korea.ORCID http://orcid.org/0000-0002-4197-9070
Soohwa JeongLow-Carbon Emission Control R&D Department, Korea Institute of Industrial Technology, Cheonan, 31056, Republic of Korea.
Ki Hyuk KangChemical & Process Technology Division, Korea Research Institute of Chemical Technology (KRICT), Daejeon, 34114, Republic of Korea.
Wangyun WonDepartment of Chemical and Biological Engineering, Korea University, Seoul, 02841, Republic of Korea. wwon@korea.ac.kr.ORCID http://orcid.org/0000-0003-1072-9842
Insoo RoDepartment of Chemical and Biological Engineering, Korea University, Seoul, 02841, Republic of Korea. insooro@korea.ac.kr.ORCID http://orcid.org/0000-0002-4704-142X

Funding

MOE | Korea Environmental Industry and Technology Institute (KEITI) 2022003650002National Research Foundation of Korea (NRF) RS-2025-24523348
6 · The paper itself

Abstract

Globally, 89% of post-consumer plastic waste is landfilled or incinerated, exacerbating environmental pollution, while less than 0.1% is chemically recycled. Polyolefin plastics, nearly half of global plastic production, can be converted into liquid fuels via hydrogenolysis or hydrocracking but require external hydrogen gas. Here, we report a tandem catalytic process combining decalin dehydrogenation with polyethylene hydrocracking, eliminating the need for external hydrogen by using decalin as a liquid organic hydrogen carrier. Among several Pt/zeolite catalysts evaluated, a bifunctional Pt/HZSM-5 catalyst is identified as the most effective, achieving high PE conversion and selectivity toward liquid fuels. Comprehensive techno-economic and life-cycle assessments are conducted for three configurations: a one-step tandem reaction that directly integrates decalin utilization, a two-step process where dehydrogenation and hydrocracking occur sequentially under hydrogen-rich conditions, and an H

Identifiers

PMID41444241
PMCPMC12830386

What OpenQuestion holds

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LicenceCC BY-NC-ND
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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.