ArticleStructural dynamics (Melville, N.Y.)2025
A UHV-compatible, time-resolved spontaneous Raman spectrometer for multi-messenger ultrafast studies: Design and applications to photoinduced dynamics.
Article in Structural dynamics (Melville, N.Y.), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Time-resolved (TR) Raman spectroscopy is a unique tool for studying the dynamic properties of quantum matter and can become a key element of the multi-messenger research in the time domain. We present here the features and results of a novel setup for TR Raman, designed to expand the NFFA-SPRINT facility by integrating it with TR optical, transient grating and electron spectroscopy and spin polarization techniques. The TR Raman setup is characterized by a wide energy tunability of the pump and probe pulses, owing to the presence of a laser system providing ultrashort (50 fs to 2 ps) light pulses from the near ultraviolet to the infrared spectral regions. The ultra-high vacuum sample environment allows for the measurement of air-sensitive samples and ensures the full compatibility with photoelectron spectroscopies, as well as a wide sample temperature range. The functionalities of the setup and the multi-messenger research approach are here demonstrated by presenting studies of the relaxation dynamics in photoexcited semiconductor systems, namely, Si and MoS
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