Evidence map›Paper›PMID 41387426›Full record

ArticleNature communications2025

Operando recombination kinetics in perovskite nanocrystal films revealed by in situ time-resolved photoluminescence.

Dandan Cao, Ziyue Jiao, Jie Gao, Yi Wang, Xi-Cheng Ai, Jian-Ping Zhang

Abstract read
In one paragraph

Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

0numbers the graph read from it
0cells of the map it votes in
1citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

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2 · The registry

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3 · Its place in the literature

Who cites it

1 citing paper in PubMed.

  1. Article
4 · The record

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5 · Who and what money

Authors and funding

6 authors.

Dandan CaoKey Laboratory of Advanced Light Conversion Materials and Biophotonics, School of Chemistry and Life Resources, Renmin University of China, Beijing, P.R. China.
Ziyue JiaoKey Laboratory of Advanced Light Conversion Materials and Biophotonics, School of Chemistry and Life Resources, Renmin University of China, Beijing, P.R. China.
Jie GaoKey Laboratory of Advanced Light Conversion Materials and Biophotonics, School of Chemistry and Life Resources, Renmin University of China, Beijing, P.R. China.
Yi WangKey Laboratory of Advanced Light Conversion Materials and Biophotonics, School of Chemistry and Life Resources, Renmin University of China, Beijing, P.R. China. ywang@ruc.edu.cn.ORCID http://orcid.org/0000-0002-8451-8629
Xi-Cheng AiKey Laboratory of Advanced Light Conversion Materials and Biophotonics, School of Chemistry and Life Resources, Renmin University of China, Beijing, P.R. China.
Jian-Ping ZhangKey Laboratory of Advanced Light Conversion Materials and Biophotonics, School of Chemistry and Life Resources, Renmin University of China, Beijing, P.R. China.

Funding

National Natural Science Foundation of China (National Science Foundation of China) 22273119National Natural Science Foundation of China (National Science Foundation of China) 22373114Natural Science Foundation of Beijing Municipality (Beijing Natural Science Foundation) 2232008
6 · The paper itself

Abstract

Perovskite nanocrystals have shown great promise for optoelectronic applications. Understanding charge recombination under operational conditions, such as continuous-wave photoexcitation, is crucial for advancing device performance. Although time-resolved photoluminescence is widely used to study recombination kinetics, its reliance on ultrafast pulsed excitation fails to replicate the operational conditions. Here we develop an integrated spectroscopy platform that enables simultaneous acquisition of steady-state and time-resolved photoluminescence under continuous-wave illumination, with a wide range of photoexcitation intensity modulation. This approach resolves the long-standing mismatch between the typical time-resolved photoluminescence data and the actual continuous-wave operational behavior of perovskite nanocrystals. In contrast to the established Auger recombination model, which suggests accelerated recombination at high pump fluence, we demonstrate that the operando recombination kinetics is governed by the charge-carrier and trap-state interaction. This clarified recombination mechanism provides insight for designing perovskite nanocrystal films applied to efficient and stable light emission under high-power photoexcitation.

Identifiers

PMID41387426
PMCPMC12728232

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