ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026
Microdroplet Stabilization Enabled Direct Mass Spectrometric Identification of Electrogenerated Transient Carbocation Intermediates.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
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Who cites it
1 citing paper in PubMed.
- Microdroplet Stabilization Enabled Direct Mass Spectrometric Identification of Electrogenerated Transient Carbocation Intermediates.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
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Authors and funding
3 authors.
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Abstract
The electrochemically generated carbocations are pivotal yet elusive intermediates in electrosynthesis. By coupling nanoelectrospray ionization with a tip-confined electrochemical microreactor, the ultrafast transfer of the electrogenerated species into the charged microdroplets is achieved. Interestingly, the highly reactive carbocations become abnormally inert in the electrosprayed microdroplets, and made a survival throughout the entire lifespans of the microdroplets. By taking full advantage of the newfangled stabilizing effect of the microdroplets, the direct mass spectrometric identification of the electrogenerated transient benzylic and phenylic carbocations, whose half-lives in bulk solutions are on the nanosecond level is achieved. The detailed paths of the carbocation-driven C(sp
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