ArticleNature communications2025
Conflicting entropy-driven zwitterionic dry polymer electrolytes for scalable high-energy all-solid-state batteries.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
What it found
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The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
5 citing papers in PubMed.
- Multiple Strong Ion-Dipole Interactions in Hierarchical Porous Polymer/Covalent Organic Framework Electrolytes Accelerating Stable and Efficient Ion Transport.Angewandte Chemie (International ed. in English) · 2026Article
- Zwitterionic Polymer Electrolytes With Dipole-Rotation-Assisted Ion Conduction for Solid Lithium Metal Batteries.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Zwitterionic Dynamic Supramolecular Elastomer Electrolytes for High-Voltage and Dendrite-Free Lithium Metal Batteries.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- MoClScience advances · 2026Article
- Charge-engineered cellulose nanofibril binders for PFAS-free, high-loading lithium battery positive electrodes.Nature communications · 2026Article
Corrections and comments
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Authors and funding
19 authors.
Funding
Abstract
Inorganic electrolytes dominate all-solid-state batteries (ASSBs), but face critical limitations, including interfacial instability, complex manufacturing, and challenges in operating under commercially viable conditions. Here, we present a transformative approach using zwitterionic dry polymer electrolytes (ZPEs) designed via a conflicting entropy strategy to enable scalable energy-dense ASSBs. Guided by Flory-Huggins theory, liquid-state zwitterionic monomers exhibit higher mixing entropy with Li salts compared to conventional long-chain polymers, forming homogeneous monomer/salt mixtures with enhanced intermolecular electrostatic interactions to promote salt dissociation. In situ polymerization of these mixtures yields directionally aligned ion channels decoupled from the polymer backbone, characterized by reduced conformational entropy, allowing rapid Li⁺ migration via an ion-hopping mechanism under ambient conditions. The ZPEs are seamlessly incorporated as a solid catholyte into pre-fabricated high-areal-capacity (10.0 mAh cm⁻²) LiNi
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Registered trials
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