Evidence map›Paper›PMID 41298435›Full record

ArticleNature communications2025

Carbon defects enhanced TEMPO redox cycles for high-efficiency urotropine electrosynthesis.

Shiyun Li, Guangsheng Liu, Chuhao Liu, Yifan Fu, Yixuan Fu, Yifei Xu, Chengyu Li, Xueqiang Zhang, Bingjun Xu, Wan-Lu Li and 1 more

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

0numbers the graph read from it
0cells of the map it votes in
1citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

1 citing paper in PubMed.

  1. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

11 authors.

Shiyun Li *Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, China.ORCID http://orcid.org/0000-0003-1240-1779
Guangsheng Liu *Program of Materials Science and Engineering, University of California San Diego, La Jolla, CA, USA.
Chuhao Liu *Institute of Molecular Engineering Plus, College of Chemistry, Fuzhou University, Fuzhou, China.
Yifan FuBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, China.
Yixuan FuBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, China.
Yifei XuBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, China.ORCID http://orcid.org/0000-0002-4331-0645
Chengyu LiBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, China.
Xueqiang ZhangLaser Micro/Nano-Fabrication Laboratory, School of Mechanical Engineering, Beijing Institute of Technology, Beijing, China. xueqiangzhangme@bit.edu.cn.
Bingjun XuBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, China. b_xu@pku.edu.cn.ORCID http://orcid.org/0000-0002-2303-257X
Wan-Lu LiProgram of Materials Science and Engineering, University of California San Diego, La Jolla, CA, USA. wal019@ucsd.edu.ORCID http://orcid.org/0000-0003-0098-0670
Mufan LiBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, China. mufanli@pku.edu.cn.ORCID http://orcid.org/0000-0002-4575-4055

Funding

National Natural Science Foundation of China (National Science Foundation of China) 22372004Natural Science Foundation of Beijing Municipality (Beijing Natural Science Foundation) Z240027
6 · The paper itself

Abstract

Electrocatalysis provides a sustainable alternative route to produce nitrogen-containing molecules. However, poor carbon-nitrogen (C-N) coupling selectivity and limited current density pose challenges to its widespread adoption. Herein, we introduce a carbon-defect enhanced 2,2,6,6-tetramethylpiperidine N-oxyl (TEMPO) mediated tandem process to tackle both problems. Our hetero-homogeneous system achieves a Faraday efficiency of ~99% with industrial-level current density of ~0.6 A·cm

Identifiers

PMID41298435
PMCPMC12657929

What OpenQuestion holds

Textmetadata
LicenceCC BY-NC-ND
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.