ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026
Sabatier-Adjusted d-Band Centers of Scalable Asymmetric Iron Sites toward Dynamic Nonradical Network for Fast Mineralization with Low-Amount Oxidant.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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Who cites it
1 citing paper in PubMed.
- Sabatier-Adjusted d-Band Centers of Scalable Asymmetric Iron Sites toward Dynamic Nonradical Network for Fast Mineralization with Low-Amount Oxidant.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
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11 authors.
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Abstract
Nonradicals relying on peroxymonosulfate (PMS) activation face inherent kinetic and thermodynamic limitations in pollutant mineralization. This is overcome using asymmetric iron single-atom catalysts (Fe-SACs) with Sabatier-adjusted d-band centers that establish a synergistic nonradical network of pathways, achieving exceptional mineralization (≈85%) with only one-tenth conventional PMS dosage. Direct coordination of high-loading Fe (≈10 wt.%) with controllable p-block elements (S, P, B) simultaneously facilitates electron-transfer pathways and selective generation of nonradicals (
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