Evidence map›Paper›PMID 41274932›Full record

ArticleNature communications2025

Understanding thermal transport in polymer semiconductors via two-channel mechanism.

Chunlin Xu, Dongyang Wang, Zhaodong Zhu, Svemir Rudić, Sihai Yang, Chong-An Di, Dong Wang

Abstract read
In one paragraph

Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Article
  2. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

7 authors.

Chunlin XuState Key Laboratory of Flexible Electronics Technology, Beijing Tsinghua Institute for Frontier Interdisciplinary Innovation, Tsinghua University, Beijing, PR China.ORCID http://orcid.org/0000-0003-4309-2307
Dongyang WangBeijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing, PR China.ORCID http://orcid.org/0009-0005-2559-1163
Zhaodong ZhuDepartment of Chemistry, University of Manchester, Manchester, UK.ORCID http://orcid.org/0000-0002-0204-8687
Svemir RudićISIS Facility, STFC Rutherford Appleton Laboratory, Oxfordshire, UK.ORCID http://orcid.org/0000-0003-3023-8565
Sihai YangCollege of Chemistry and Molecular Engineering, Beijing National Laboratory for Molecular Sciences, Peking University, Beijing, PR China.
Chong-An DiBeijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing, PR China.ORCID http://orcid.org/0000-0002-6183-1321
Dong WangState Key Laboratory of Flexible Electronics Technology, Beijing Tsinghua Institute for Frontier Interdisciplinary Innovation, Tsinghua University, Beijing, PR China. dong913@tsinghua.edu.cn.ORCID http://orcid.org/0000-0002-0594-0515

Funding

National Natural Science Foundation of China (National Science Foundation of China) 22273043
6 · The paper itself

Abstract

The vibrational thermal conductivity of polymer semiconductors is critical to the performance of organic electronic devices, yet its underlying mechanisms remain elusive. This work presents a two-channel model to elucidate the vibrational heat transport in semiconducting polymers with extended side chains. We reveal a striking splitting of vibrational modes along the polymer chain, driven by the substantial difference in force constants between the backbone and side chains. This gives rise to two distinct dispersive longitudinal branches: a backbone branch, characterized by phonon-like propagons that govern thermal conductivity, and a side chain branch, consisting of non-propagating diffusons that make minimal contributions to heat transport. The reduced maximum thermal conductivity of these polymer semiconductors, compared to their side chain-free counterparts, is attributed to phonon scattering by the low-frequency optical modes of the side chains. Our findings establish a foundation for strategically modifying side chains as a potent approach to fine-tuning thermal conductivity.

Identifiers

PMID41274932
PMCPMC12749816

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.