ArticleScience advances2025
High-strength and fracture-resistant ionogels via solvent-tailored interphase cohesion in nanofibrous composite networks.
Article in Science advances, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Tailored construction and functional applications of conductive hydrogels for bioelectronic interfaces.Discover nano · 2026Review
- One-dimensional architectures in polymer solid electrolytes: design principles, ion-transport mechanisms and practical implementation.Chemical science · 2026Review
- Cellulose Ionogels: Unraveling Structure-Property Relationships Through Multiscale In-Situ Characterization and Theoretical Modeling.Gels (Basel, Switzerland) · 2026Review
- Bio-Ionic Liquid-Induced Rapid Self-Initiating Tough Ionogels for In Situ Adhesion.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Recent Advances in Polypyrrole-Based Functional Coatings: Surface Protection and Emerging Applications.Materials (Basel, Switzerland) · 2026Review
- Interfacial Engineering for High-Output, Mechanically Robust Fully Stretchable Moisture-Electric Generators.Nano-micro letters · 2026Article
- A 10-micrometer-thick hydrogel membranes for robust and conformal bioelectronic interfaces.National science review · 2026Article
- Ultrathin and ultrastrong hydrogel bioelectronic membranes.National science review · 2026Article
- EGaIn-Activated Bioinspired Silk Micro/Nanofibril Eutectogels Breaking the Strength-Conductivity Trade-Off for High-Performance Wearable Bioelectronics.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
Corrections and comments
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Authors and funding
9 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Ionogels are promising for soft robotics, energy systems, and bioelectronic interfaces due to their high ionic conductivity and environmental stability. However, combining high strength and fracture resistance remains challenging. Here, we report composite ionogels with outstanding mechanical strength (~65.4 megapascal) and fracture energy (~607 kilojoules per square meter), capable of bearing more than 5000 times their own weight. These ionogels are developed by tailoring solvent-solute interactions to create a dense, hyperconnected nanofibrous polymer network. Solvent engineering regulates hydrogen bonding competition, facilitating the formation of robust interphase hydrogen bonds and a soft-hard biomimetic interface. Moreover, their antidrying, breathable nature enables multifunctional electrophysiological monitoring, making them ideal for wearable bioelectronics. Their ionic conductivity, drug-loading capacity, and antibacterial properties allow their use in advanced e-bandages for chronic wound healing. This generalizable strategy for ionogel design opens pathways toward strong, versatile, and biocompatible materials, particularly valuable for next-generation soft materials, wearable electronics, and tissue engineering.
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Registered trials
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