Evidence map›Paper›PMID 41255185›Full record

ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026

Deuteration Induced Electron-Phonon Coupling Modulation: Suppressing Energy Dissipation and Enhancing Carrier Separation in Organic Photocatalysis.

Hongli Sun, Zirui Zhou, Yunfei Ma, Qingzhu Xu, Yanglong Liao, Cheng Han, Yue Zheng, Xiaosong Cao, Yu Wang, Zutao Fan and 4 more

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Article
  2. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

14 authors.

Hongli SunInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Zirui ZhouInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Yunfei MaInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Qingzhu XuInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Yanglong LiaoInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Cheng HanInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Yue ZhengInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Xiaosong CaoShenzhen Key Laboratory of New Information Display and Storage Materials, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518060, China.
Yu WangInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Zutao FanInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Jianfeng ZhaoState Key Laboratory of Catalysis, Dalian National Laboratory for Clean Energy, The Collaborative Innovation Centre of Chemistry for Energy Materials (iChEM), Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, 116023, China.
Chenliang SuInternational Collaboration Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University, Shenzhen, 518060, China.
Fengtao FanState Key Laboratory of Catalysis, Dalian National Laboratory for Clean Energy, The Collaborative Innovation Centre of Chemistry for Energy Materials (iChEM), Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, 116023, China.
Bin LiuDepartment of Materials Science and Engineering, City University of Hong Kong, Hong Kong SAR, 999077, China.ORCID https://orcid.org/0000-0002-4685-2052

Funding

China Postdoctoral Science Foundation 2023M742395City University of Hong Kong 9020003Graduate Student Innovation Incubator Program of Shenzhen University 868-000002020269Guangdong Basic and Applied Basic Research Foundation 2020A1515010982ITF-RTH-Global STEM Professorship 9228005ITF-RTH-Global STEM Professorship 9446006JC STEM lab of Advanced CO2 Upcycling 9228005National Key Research and Development Program of China 2021YFA1600800National Key Research and Development Program of China 2023YFA1507003National Natural Science Foundation of China 22101185National Natural Science Foundation of China 22102102National Natural Science Foundation of China 22302191National Natural Science Foundation of China 22372102National Natural Science Foundation of China 22402122National Natural Science Foundation of China 62275162Research Team Cultivation Program of Shenzhen University 2023QNT013Scientific Foundation for Youth Scholars of Shenzhen University 868-000001032185Shenzhen Peacock Plan 20210308299CShenzhen Science and Technology Program 20231121175024001Shenzhen Science and Technology Program 20231122120657001Shenzhen Science and Technology Program JCYJ20241202124510014Shenzhen Science and Technology Program RCJC20200714114434086
6 · The paper itself

Abstract

The electron-phonon coupling in organic photocatalysts offers a great opportunity for tuning carrier behaviors and energy dissipation toward improving photocatalytic efficiency. Adopting strategies to tailor electron-phonon coupling and revealing the underlying mechanism are therefore essential for the development of high-efficiency organic photocatalysts. In this work, an isotope substitution strategy is developed by replacing H in high-frequency C─H oscillators with D to tune the electron-phonon coupling strength of both 1,2,3,5-tetrakis(carbazol-9-yl)-4,6-dicyanobenzene (4CzIPN) and its polymeric derivative. The fitted Huang-Rhys factors exhibit an ≈1.7-fold increase upon isotopic deuteration, revealing enhanced electron-phonon coupling. Comprehensive studies demonstrate that the deuteration strategy can effectively lower exciton binding energy, promote exciton dissociation, and suppress non-radiative energy dissipation, therefore leading to an improved efficiency toward photocatalytic hydrogen evolution. This study highlights the crucial role of electron-phonon coupling on photocatalytic systems and presents a novel regulatory strategy for designing high-efficiency organic photocatalysts.

Indexed as

4CzIPNdeuterationelectron‐phonon couplingnon‐radiative energy dissipationorganic photocatalysts

Identifiers

PMID41255185
PMCPMC12866818

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.