ArticleACS materials Au2025
Encapsulation Strategy Matters: Pre- and Post-Loading of Macromolecules into Surface-Supported Microgels Formed via Vaterite Templates.
Article in ACS materials Au, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Calcium carbonate vaterite crystals have attracted increasing attention as sacrificial templates for forming polymer microgels. Vaterite's porous structure, biocompatibility, and eco-friendly synthesis make it ideal for biomedical applications. In this study, vaterite is grown on the surface, and surface-supported (ss)-microgels are formed by coating it with alternating layers of polyelectrolytes, sodium alginate (ALG), and poly-l-lysine (PLL), followed by core dissolution. Pre-loading (during vaterite synthesis) and post-loading (after microgel formation) of macromolecules are compared using dextran and its charged derivatives. Pre-loading proved to be more efficient, achieving up to 9% w/w encapsulation. Dextran adsorption follows the Langmuir model (Δ
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