ArticleRSC advances2025
Cyclodextrin-threaded covalent organic polyrotaxanes with tunable solid-state emissive activity for efficient iodine capture.
Article in RSC advances, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Herein, we rationally designed and synthesized a covalent organic polyrotaxane (COPR), with aggregation-induced emission (AIE) characteristics, denoted as TPE-CD-COPR, through a two-component Knoevenagel condensation reaction, where β-cyclodextrin (β-CD) inclusion complexes served as direct building blocks. This approach yielded several remarkable improvements over conventional CD-free counterpart (TPE-COP). The threading of CD not only achieved precise tuning of solid-state emission color under UV irradiation, but also introduced significant polarity enhancement through rotaxane subunit incorporation. The incorporation of water-soluble cyclodextrin rotaxane architectures significantly enhanced the aqueous dispersibility, thereby providing an optimal solution for developing high-performance aqueous-phase iodine adsorbents. As a result, TPE-CD-COPR demonstrated significantly enhanced aqueous-phase iodine adsorption capabilities, exhibiting both superior capacity and faster kinetics compared to conventional CD-free counterpart. The enhanced I
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