ArticleChemSusChem2025
Unveiling the Electrochemical Reversibility of Multielectron Redox in s-Tetrazine Derivatives for Large-Capacity Electrode Materials.
Article in ChemSusChem, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.
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Who cites it
2 citing papers in PubMed.
- Guest-Dependent Fluorescence Response by a Highly Emissive s-Tetrazine PdChemistry, an Asian journal · 2026Article
- Unveiling the Electrochemical Reversibility of Multielectron Redox in s-Tetrazine Derivatives for Large-Capacity Electrode Materials.ChemSusChem · 2025Article
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Authors and funding
4 authors.
Funding
Abstract
1,2,4,5-tetrazine (s-tetrazine) is a promising redox center for organic electrode materials due to its low molecular weight and ability to undergo two-electron redox reactions. However, in practice, the irreversibility of the second-electron transfer has often limited the specific capacities of the s-tetrazine-based electrodes in metal-organic cells. Herein, electrochemically reversible two-electron-transfer processes from the s-tetrazine core are demonstrated by introducing electron-withdrawing pyridine rings at 3- and 6-positions. Comparative analysis of three s-tetrazine derivatives, 3,6-diphenyl-1,2,4,5-tetrazine (Ph-Tz), 3,6-di(4-pyridinyl)-1,2,4,5-tetrazine (4-Py-Tz), and 3,6-di(2-pyridinyl)-1,2,4,5-tetrazine (2-Py-Tz) reveals that both electron-withdrawing effect and Li-ion coordination play critical roles in redox reversibility. Among them, 2-Py-Tz exhibits the highest electron-transfer rate with Li
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