ArticleNano letters2025
Singlet Fission Luminescent Solar Concentrators.
Article in Nano letters, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Authors and funding
10 authors.
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Abstract
Luminescent solar concentrators (LSCs) present a promising avenue for solar energy harvesting, utilizing transparent matrices embedded with light-absorbing chromophores to concentrate incident solar radiation. Photon-multiplier luminescent solar concentrators (PM-LSCs) contain chromophores boasting over 100% photoluminescence quantum efficiency. Although PM-LSCs may bypass free energy losses observed in traditional LSC systems, experimental PM-LSCs have exhibited optical efficiency sensitivity to photon flux. Here, we demonstrate a PM-LSC utilizing singlet fission (SF), an exciton multiplication process. We apply large-area films of absorbing TIPS-tetracene mixed with tetracene-carboxylic acid-ligated PbS quantum dots and demonstrate they are suitable for solid-state LSC devices. We find that although SF-LSCs present pathways to mitigate fluence limitations observed in quantum cutting systems, challenges persist due to triplet-triplet annihilation (TTA) at higher photon fluxes. The potential of SF-LSCs to overcome fluence limitations in PM-LSCs suggests a promising avenue for future development.
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