Evidence map›Paper›PMID 41168213›Full record

ArticleNature communications2025

Kinetically-controlled intermediate-direct-pinning for homogeneous energy landscapes in quasi-two-dimensional perovskites for efficient and narrow blue emission.

Joo Sung Kim, Hyeon-Dong Lee, Jeong Hyun Jung, Taehee Kim, Seung-Je Woo, Hyung Joong Yoon, Jaehyun Moon, Chan-Mo Kang, Seung-Eui Chang, Dong-Hyeok Kim and 4 more

Abstract read
In one paragraph

Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.

0numbers the graph read from it
0cells of the map it votes in
3citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

3 citing papers in PubMed.

  1. Review
  2. Article
  3. Review
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

14 authors.

Joo Sung Kim *Department of Materials Science and Engineering, Seoul National University, 1 Gwanak-ro Gwanak-gu, Seoul, Republic of Korea.ORCID http://orcid.org/0000-0002-7465-3085
Hyeon-Dong Lee *Department of Materials Science and Engineering, Seoul National University, 1 Gwanak-ro Gwanak-gu, Seoul, Republic of Korea.
Jeong Hyun Jung *Department of Materials Science and Engineering, Seoul National University, 1 Gwanak-ro Gwanak-gu, Seoul, Republic of Korea.ORCID http://orcid.org/0000-0002-2043-6595
Taehee Kim *Department of Chemistry, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, Republic of Korea.ORCID http://orcid.org/0000-0001-9426-1006
Seung-Je WooDepartment of Materials Science and Engineering, Seoul National University, 1 Gwanak-ro Gwanak-gu, Seoul, Republic of Korea.ORCID http://orcid.org/0000-0001-7364-7479
Hyung Joong YoonResearch Center for Materials Analysis, Korea Basic Science Institute (KBSI), 169-148 Gwahak-ro, Yuseong-gu, Daejeon, Republic of Korea.
Jaehyun MoonReality Devices Research Division, Electronics and Telecommunications Research Institute, 218, Gajeong-ro, Yuseong-gu, Daejeon, Republic of Korea.
Chan-Mo KangReality Devices Research Division, Electronics and Telecommunications Research Institute, 218, Gajeong-ro, Yuseong-gu, Daejeon, Republic of Korea.ORCID http://orcid.org/0000-0001-7246-3731
Seung-Eui ChangDepartment of Materials Science and Engineering, Seoul National University, 1 Gwanak-ro Gwanak-gu, Seoul, Republic of Korea.ORCID http://orcid.org/0009-0004-5554-0626
Dong-Hyeok KimDepartment of Materials Science and Engineering, Seoul National University, 1 Gwanak-ro Gwanak-gu, Seoul, Republic of Korea.
Sungjin KimDepartment of Materials Science and Engineering, Seoul National University, 1 Gwanak-ro Gwanak-gu, Seoul, Republic of Korea.ORCID http://orcid.org/0000-0001-7146-5479
Hoichang YangDepartment of Chemical Engineering, Inha University, 100 Inha-ro, Michuhol-gu, Incheon, Republic of Korea.
Dongho KimDepartment of Chemistry, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, Republic of Korea. dongho@yonsei.ac.kr.ORCID http://orcid.org/0000-0001-8668-2644
Tae-Woo LeeDepartment of Materials Science and Engineering, Seoul National University, 1 Gwanak-ro Gwanak-gu, Seoul, Republic of Korea. twlees@snu.ac.kr.ORCID http://orcid.org/0000-0002-6449-6725

Funding

National Research Foundation of Korea (NRF) 2021R1A2C300630813National Research Foundation of Korea (NRF) 2022H1D3A3A01081288
6 · The paper itself

Abstract

Quasi-two-dimensional perovskite structures hold great potential as active layers in blue perovskite light-emitting diodes. However, they face challenges of limited emission efficiency and broadened spectra due to phase inhomogeneity. Here, we report an intermediate-direct-pinning method to develop a uniform-phase quasi-two-dimensional structure with a homogeneous energy landscape. By forming a strong cation-π interaction complex, we stabilize a metastable intermediate phase with retarded crystallization toward low-n phases (n ≤ 3), followed by a direct pinning process favouring crystallization of medium-n phases (n = 4 and 5) without further broadening. Additionally, introducing a surface-anchoring ligand during the pinning process effectively suppresses non-radiative recombination. The resultant structure shows efficient sky-blue emission and narrow linewidth (108 meV). Devices fabricated with this structure reach a maximum external quantum efficiency of 22.5% at 489 nm, which is scalable to large-area (pixel size: 900 mm

Identifiers

PMID41168213
PMCPMC12575853

What OpenQuestion holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.