ArticleNature communications2025
Counter-propagating entangled photon pairs from monolayer GaSe.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
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3 citing papers in PubMed.
- Polariton spectroscopy at the diamond K-edge via X-ray parametric down-conversion.Scientific reports · 2026Article
- In-line fiber-integrated photon-pair generation from van der Waals crystals.Nano convergence · 2026Article
- Simultaneous Type-0 and Type-I Optical Parametric Oscillation in Submicron Poled Thin-Film Lithium Niobate.Nanophotonics (Berlin, Germany) · 2026Article
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12 authors.
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Abstract
Non-phase-matched spontaneous parametric down-conversion (SPDC) in atomically thin materials provides new degrees of freedom and enhanced quantum information capacity compared to conventional phase-matched sources. These systems emerged as promising platforms for quantum computing, communication, and imaging, with the potential to support higher-order nonlinear processes. However, direct observation of photon-pair emission from a monolayer has remained experimentally challenging. In this work, we theoretically modeled SPDC emission across the full angular space from a monolayer GaSe film and experimentally validated the model through measurements of both co- and counter-propagating photon pairs. We demonstrated two-photon quantum correlations in the telecom C-band from a monolayer SPDC source. The spatially symmetric, broadband emission predicted by theory was confirmed experimentally. Furthermore, we observed high-fidelity Bell states in the counter-propagating configuration. Our results revealed the emission characteristics of SPDC in the deeply subwavelength, non-phase-matched regime, and introduced atomically thin, counter-propagating SPDC as a scalable and integrable platform for programmable quantum state generation, extendable via moiré superlattice engineering.
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