ArticleJournal of the American Chemical Society2025
A Heterogenized Molecular Catalyst for the Gas-Phase Cyclotrimerization of Acetylene to Benzene.
Article in Journal of the American Chemical Society, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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8 authors.
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Abstract
Facilitating the cyclotrimerization of acetylene to benzene in the gas-phase on the surface of solid catalysts has captivated researchers, both theoretically and experimentally, for several decades. Coupled with acetylene production from renewable feedstocks, this reaction offers a promising pathway for the direct, low-temperature synthesis of renewable benzene. Recognizing the physical limitations of typical solid catalysts, which adsorb benzene too strongly, this study investigates various high-valent early transition metal chlorides─potent molecular cyclotrimerization catalysts─as solid catalysts in this gas-phase conversion. Alongside catalytic assessment under industrially relevant conditions, various analytical techniques such as
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