ArticleNature communications2025
Light-induced pressurization effect in Au-Ni heterostructures for plasmonic photocatalysis.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
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Authors and funding
13 authors.
Funding
Abstract
Plasmonic photocatalysis offers a promising route to harvest solar energy and drive chemical reactions by the generated heat and energetic charge carriers towards a low-carbon economy. Understanding the mechanisms of plasmonic photocatalysis is vital for the rational design of efficient catalysts but remains a great challenge. Here we report the discovery of an overlooked photocatalytic mechanism based on the enhanced coverage of CO on an Au-Ni heterostructure under light. Detailed studies reveal that hot carrier transfer from Au to Ni via plasmonic excitation increases the electron density of Ni, thereby boosting the population of Ni sites capable of CO adsorption. This increase in active CO-binding sites, rather than local heating or altered adsorption properties of individual Ni sites, is found to be the major contributor to the light-promoted CH
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