Bioinspired synergistic texture and color modulation enabled by surface instability of cholesteric liquid crystal elastomer bilayers.

Certain cephalopods can dynamically camouflage by altering both skin texture and color to match their surroundings. Inspired by this capability, we present a cholesteric liquid crystal elastomer-liquid crystal elastomer (CLCE-LCE) bilayer capable of simultaneous, reversible modulation of surface texture and structural color through programmable wrinkling. By tuning the bilayer's fabrication parameters, on-demand wrinkle morphologies and color combinations are achieved. Spatially selective ultraviolet (UV) curing allows localized surface textures, while chemical patterning of the CLCE layer enables region-specific color responses, expanding the design space for multifunctional, spatially encoded optical materials. The CLCE-LCE bilayer enables dynamic thermal regulation by tuning light absorption through synergistically modulating surface morphology and color. Notably, this system achieves strain-dependent multistate encoding via multistep selective UV curing, revealing distinct visual content under different applied strains. This work establishes a versatile platform that merges surface instabilities with tunable structural coloration, advancing intelligent materials with programmable, strain-responsive surface and optical properties.