Evidence map›Paper›PMID 41125574›Full record

ArticleNature communications2025

Decoding single-crystal lithium growth through solid electrolyte interphase omics.

Gongxun Lu, Zhiyuan Han, Lei Shi, Zhilong Wang, Mengtian Zhang, Xinru Wu, Zhihong Piao, Xiao Xiao, Shengyu Tao, Jianwei Nai and 8 more

Abstract read
In one paragraph

Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.

0numbers the graph read from it
0cells of the map it votes in
7citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

7 citing papers in PubMed.

  1. Review
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

18 authors.

Gongxun Lu *Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China. gongxunlu@cjlu.edu.cn.ORCID http://orcid.org/0000-0003-3490-393X
Zhiyuan Han *Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China.
Lei Shi *National Key Laboratory of Advanced Micro and Nano Manufacture Technology, Shanghai Jiao Tong University, Shanghai, China.
Zhilong WangNational Key Laboratory of Advanced Micro and Nano Manufacture Technology, Shanghai Jiao Tong University, Shanghai, China.ORCID http://orcid.org/0000-0002-1910-3654
Mengtian ZhangTsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China.
Xinru WuTsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China.
Zhihong PiaoTsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China.
Xiao XiaoTsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China.
Shengyu TaoTsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China.ORCID http://orcid.org/0000-0001-5249-432X
Jianwei NaiCollege of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, China.ORCID http://orcid.org/0000-0001-9681-5498
Zhijin JuCollege of Chemistry and Materials Engineering, Wenzhou University, Wenzhou, Zhejiang, China.ORCID http://orcid.org/0000-0003-1537-5393
Xuan ZhangTsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China.ORCID http://orcid.org/0000-0002-7537-4002
Yanqiang HanNational Key Laboratory of Advanced Micro and Nano Manufacture Technology, Shanghai Jiao Tong University, Shanghai, China.ORCID http://orcid.org/0000-0001-5454-0617
Karl Luigi Loza VidaurreNational Key Laboratory of Advanced Micro and Nano Manufacture Technology, Shanghai Jiao Tong University, Shanghai, China.ORCID http://orcid.org/0009-0003-9629-3652
Hongyan FuTsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China.ORCID http://orcid.org/0000-0002-4276-0011
Jinjin LiNational Key Laboratory of Advanced Micro and Nano Manufacture Technology, Shanghai Jiao Tong University, Shanghai, China. lijinjin@sjtu.edu.cn.ORCID http://orcid.org/0000-0003-4661-4051
Xinyong TaoCollege of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, China. tao@zjut.edu.cn.ORCID http://orcid.org/0000-0003-4084-7743
Guangmin ZhouTsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, China. guangminzhou@sz.tsinghua.edu.cn.ORCID http://orcid.org/0000-0002-3629-5686

Funding

National Science Foundation of China | NSAF Joint Fund U21A20174
6 · The paper itself

Abstract

Accurately understanding the impact of solid electrolyte interphase (SEI) on lithium deposition is critical for high-energy lithium metal batteries. Yet traditional strategies, focusing solely on isolated components, fail to capture multi-constituent synergies and underlying mechanisms. To address this challenge, we introduce the concept of SEI omics and establish a dataset of cryogenic transmission electron microscopy images combined with co-localized component information. By integrating interpretable machine learning and physics-based feature selection, we decoupled the roles of SEI constituents, revealing that higher N/S/P/F content and reduced O in the SEI improve lithium deposition. Combined density functional theory and electrochemical phase-field modeling uncovered multi-scale effects of SEI components on Li growth. Results confirm that designing an inner SEI layer with high surface energy and migration ability significantly refines deposition morphology. Guided by machine learning-optimized composition, a highly disordered SEI was engineered, achieving high average Coulombic efficiency of 99.35% over 800 cycles for Li||Cu cell at 1 mA cm

Identifiers

PMID41125574
PMCPMC12546825

What OpenQuestion holds

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Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.