ArticleSmall (Weinheim an der Bergstrasse, Germany)2025
Composition Dependent Dynamic Behaviors of Non-Stoichiometric Cocrystalline Hydrogen-Bonded Organic Frameworks.
Article in Small (Weinheim an der Bergstrasse, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
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3 citing papers in PubMed.
- Detection and Capture of Volatile Fluorinated Compounds Using Porous Materials.Nanomaterials (Basel, Switzerland) · 2026Review
- Rapidly Diversifying Hydrogen-Bonded Organic Frameworks With Permanent Porosity.Angewandte Chemie (International ed. in English) · 2026Review
- Composition Dependent Dynamic Behaviors of Non-Stoichiometric Cocrystalline Hydrogen-Bonded Organic Frameworks.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
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Abstract
Non-stoichiometric multicomponent crystals have the potential not only to fine-tune material properties but also to emerge new functionalities. In this paper, the composition-dependent dynamic transformation of non-stoichiometric cocrystalline hydrogen-bonded organic frameworks (NS-HOFs) composed of tetrakis(4-carboxyphenyl)hexahydropyrene and -pyrene derivatives (CP-Hp and CP-Py, respectively) is reported. Isostructural mono-component frameworks of CP-Hp and CP-Py (CP-Hp-1 and CP-Py-1, respectively) underwent structural transformation into the corresponding shrunk frameworks (CP-Hp-2 and CP-Py-2, respectively) by spontaneous release of the included solvent molecules, where the transformation speed of CP-Hp-1 is faster than that of CP-Py-1. NS-HOFs of CP-Hp and CP-Py, denoted by CP-HpPy-1(x), where x is the mixing ratio of CP-Hp, show the transformation into CP-HpPy-2(x), and the transformation behaviors strongly depend on the composition ratio. Interestingly, the transformation speed is not proportional to the composition ratio, while the maximum speed is observed for CP-HpPy-1(0.5). This is, to the best of these knowledge, the first example of composition-dependent structural changes in non-stoichiometric cocrystalline frameworks, demonstrating that dynamic behaviors can be modulated nonlinearly by the composition of the frameworks and shedding light on new aspects of porous soft crystals.
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