ArticleJournal of the American Chemical Society2025
Iridium-Catalyzed Twofold C-H/C-H Activation and Annulation: Access to Anti-Kasha Emission and Photosensitive-Phosphorescent Materials.
Article in Journal of the American Chemical Society, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
The first example of a multifunctional anti-Kasha emission-photosensitive-phosphorescent material has been synthesized via an efficient twofold C-H/C-H activation and annulation protocol. Both experimental data and theoretical calculations have validated the anti-Kasha emission property of phenothiazinium and phenoxazinium salts. Specifically, the anti-Kasha emission property of phenoxazinium salts enables dual-channel emission intensity ratio imaging for visualizing cellular and intercellular structures, while also endowing them with the capability to specifically target mitochondria in living cells. Furthermore, these newly developed photosensitive-phosphorescent materials have been demonstrated to act as efficient photocatalysts in C-H bond functionalization reactions. In addition, the novel phenothiazinium salts demonstrate photosensitive and phosphorescent properties in PVA (poly(vinyl alcohol)) films: upon light irradiation, they undergo a significant blue shift accompanied by ultralong room-temperature phosphorescence, making them highly promising for applications in encryption and multichannel information storage.
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