ArticleACS polymers Au2025
Synergistic Engineering of Pyrene-Thiazolothiazole-Based Donor-π-Acceptor Conjugated Microporous Polymers with Heteroatom Embedding for Efficient Visible-Light Photocatalyst for Organic Dye Degradation.
Article in ACS polymers Au, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Water pollution caused by organic dyes poses a significant threat to ecosystems and human health, underscoring the urgent need for sustainable degradation methods. We report two donor-π-acceptor conjugated microporous polymers (CMPs), Pyr-Ph-TzTz and Pyr-Th-TzTz, assembled from pyrene (Pyr) donors, phenyl or thiophene π-bridges, and thiazolothiazole (TzTz) acceptors. Precursors [4,4',4″,4‴-(pyrene-1,3,6,8-tetrayl)-tetrabenzaldehyde (Pyr-Ph-4CHO) and 5,5',5″,5‴-(pyrene-1,3,6,8-tetrayl)-tetrakis-(thiophene-2-carbaldehyde) (Pyr-Th-4CHO)] were synthesized via electrophilic bromination and Suzuki-Miyaura coupling with 4-formylphenylboronic acid (PFPBA), and 5-formyl-2-thienylboronic acid (5-FTBA); respectively. Pyr-Ph-4CHO and Pyr-Th-4CHO were each subjected to a one-pot condensation reaction with dithiooxamide, yielding robust, thermally stable CMPsPyr-Ph-TzTz and Pyr-Th-TzTzwith amorphous frameworks and surface areas of 37 and 20 m
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