A Large-Area Uniform Three-Dimensional Covalent Organic Framework Membrane for Stabilizing Li-Metal Electrodes via Solvation Cages.

Zhuozhuo Tang, Jia Chen, Da Zhu, Li Sheng, Yang Yang, Kai Yang, Jianlong Wang, Yaping Tang, Xiangming He, Hong Xu

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Article in Research (Washington, D.C.), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

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5 · Who and what money

Authors and funding

10 authors.

Zhuozhuo TangInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.

Jia ChenInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.

Da ZhuInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.

Li ShengInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.

Yang YangInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.

Kai YangInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.

Jianlong WangInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.

Yaping TangInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.

Xiangming HeInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.

Hong XuInstitute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, P. R. China.ORCID https://orcid.org/0000-0001-7918-1454

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Covalent organic frameworks (COFs), known for their ordered structures, hold promise as ion-conducting materials in cells/batteries. Nevertheless, the rigid cross-linking of porous materials prevents them from being processed into membranes, while composite membranes weaken the material's conductivity advantage due to phase interruptions. Here, we report a phase-continuous 3-dimensional COF (3D-COF) membrane with a large size of 15 cm × 25 cm, fabricated via in situ interfacial engineering. The COF membranes possessed a non-interpenetrating dia topology that facilitated 3D continuous ionic pathways at the molecular level. Further, the hydroxyl and imine groups on the framework could form Li

Identifiers

PMID41079671

DOI10.34133/research.0926

PMCPMC12508527

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LicenceCC BY

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.