ArticleACS omega2025
Hydrophobic Eutectic Solvents for Sustainable Bisphenol A Extraction from Water: Screening and Selection Based on Key Performance Criteria.
Article in ACS omega, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Authors and funding
10 authors.
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Abstract
Hydrophobic Eutectic Solvents (HES) are emerging as a promising class of sustainable solvents for water treatment applications, yet their rational selection and performance evaluation remain limited. In this work, we adopted a systematic approach to rank a diverse set of HES, combining terpenes, fatty acids, and trioctylphosphine oxide (TOPO). The screening was based on seven key criteriaviscosity, density, water leaching, pH shift, water uptake, EcoScale score, and chemical stabilityaimed at identifying systems with low cross-contamination, high processability, and favorable environmental profiles. Selected HES were then evaluated in liquid-liquid extraction (LLE) using bisphenol A (BPA) as a model compound, with performance assessed via UV-Vis and NMR spectroscopy. The optimized HES, TOPO:menthol, demonstrated an excellent extraction efficiency and very low leaching. Reusability was explored as well as regeneration through back-extraction. Sustainability assessments using the Analytical EcoScale and AGREEprep tools reinforced the viability of the proposed systems. Beyond pollutant removal, this work offers a framework for the molecular-level design and evaluation of HES, advancing their integration into green separation technologies.
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Registered trials
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