Evidence map›Paper›PMID 41038873›Full record

ArticleNature communications2025

Facile cascade-anchored synthesis of ultrahigh metal loading single-atom for significantly improved Fenton-like catalysis.

Shuaishuai Li, Wei Wang, Huizhong Wu, Xuechun Wang, Shihu Ding, Jingyang Liu, Xiuwu Zhang, Jiangli Sun, Chunhong Fu, Minghua Zhou

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

0numbers the graph read from it
0cells of the map it votes in
1citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

1 citing paper in PubMed.

  1. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

10 authors.

Shuaishuai LiMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China.
Wei WangMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China. nkwangwei@126.com.
Huizhong WuMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China.
Xuechun WangMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China.
Shihu DingMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China.
Jingyang LiuMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China.
Xiuwu ZhangMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China.
Jiangli SunMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China.
Chunhong FuMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China.
Minghua ZhouMOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution, College of Enviromental Science and Engineering, Nankai University, Tianjin, China. zhoumh@nankai.edu.cn.ORCID http://orcid.org/0000-0003-1306-3505

Funding

National Natural Science Foundation of China (National Science Foundation of China) U23B20165
6 · The paper itself

Abstract

It is crucial to break the low metal-loading limitation and reveal the intersite synergy-governed catalytic behavior of single-atom catalysts (SACs). Here, a universal synthesis strategy achieves record loadings of transition metals (Fe 41.31 wt%, Mn 35.13 wt%), rare-earth metals (La 28.62 wt%), and noble metals (Ag 27.04 wt%). The strong oxalic acid-metal chelation and concurrent entangled polymer networks enable high-loading SACs. High-density single atoms induce site-intensive effects, modulating electron density and valence states to achieve peroxymonosulfate-based Fenton-like reactions with rate constants 1-2 orders of magnitude higher than conventional SACs. Elevated metal loading boosts Fenton-like potential jumps, facilitates electron transfer, and reduces the rate-limiting energy barrier in

Identifiers

PMID41038873
PMCPMC12491624

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.