Evidence map›Paper›PMID 41038836›Full record

ArticleNature communications2025

Leveraging catechol chemistry to tackle toughness-softness-work capacity tradeoff in reprogrammable liquid crystal actuators.

Enjian He, Yahe Wu, Huan Liang, Hongtu Xu, Jiujiang Ji, Zhijun Yang, Yixuan Wang, Yen Wei, Yan Ji

Abstract read
In one paragraph

Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Article
  2. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

9 authors.

Enjian HeThe Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology (Ministry of Education), Department of Chemistry, Tsinghua University, Beijing, China.
Yahe WuSchool of Chemistry and Chemical Engineering, Beijing Institution of Technology, Beijing, China. wuyahe0603@bit.edu.cn.ORCID http://orcid.org/0000-0003-4740-9447
Huan LiangThe Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology (Ministry of Education), Department of Chemistry, Tsinghua University, Beijing, China.ORCID http://orcid.org/0009-0000-2511-8310
Hongtu XuThe Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology (Ministry of Education), Department of Chemistry, Tsinghua University, Beijing, China.
Jiujiang JiThe Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology (Ministry of Education), Department of Chemistry, Tsinghua University, Beijing, China.
Zhijun YangThe Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology (Ministry of Education), Department of Chemistry, Tsinghua University, Beijing, China.
Yixuan WangThe Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology (Ministry of Education), Department of Chemistry, Tsinghua University, Beijing, China.
Yen WeiDepartment of Chemistry, Center for Nanotechnology and Institute of Biomedical Technology, Chung-Yuan Christian University, Taiwan, China.ORCID http://orcid.org/0000-0001-5950-0163
Yan JiThe Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology (Ministry of Education), Department of Chemistry, Tsinghua University, Beijing, China. jiyan@mail.tsinghua.edu.cn.ORCID http://orcid.org/0000-0002-1363-6513

Funding

National Natural Science Foundation of China (National Science Foundation of China) 21788102National Natural Science Foundation of China (National Science Foundation of China) 22375114National Natural Science Foundation of China (National Science Foundation of China) 52303089
6 · The paper itself

Abstract

Dynamic chemistry endows liquid crystal elastomers (LCEs) with reprogrammability, enabling the reversible modulation of actuation modes to adapt to diverse tasks and enhancing sustainability and lifecycle management. However, balancing toughness, softness, and work capacity remains challenging due to their inherent tradeoff, as these properties are essential for achieving high-performance and stable actuation. Here, inspired by mussel coordination chemistry, we design a macromolecular crosslinker that combines covalent crosslinking with coordination bonds to tackle this challenge. The optimized LCE achieves exceptional toughness of 28.5 MJ/m³ and low Young's modulus of 3.1 MPa, with high-temperature toughness exceeding 9.3 MJ/m³ at 90 °C (25 °C above phase transition temperature, T

Identifiers

PMID41038836
PMCPMC12491623

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.