ArticleNature chemistry2025
Electrifying industrial hydrogen peroxide production via soft interfacial molecular mediation.
Article in Nature chemistry, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
What it found
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The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
7 citing papers in PubMed.
- Design and Modulation of Oxygen Vacancy-Rich Catalysts for Hydrogen and Oxygen Electrocatalysis in Energy Conversion.Small (Weinheim an der Bergstrasse, Germany) · 2026Review
- Unassisted bipolar photoelectrochemical synthesis of HNature communications · 2026Article
- Calcium-tolerant electrode strategy for efficient hydrogen peroxide electrosynthesis in natural water.Nature communications · 2026Article
- Membrane-Confined Proton Management Orchestrates Proton-Electron Transfer for Efficient Photocatalytic Hydrogen Peroxide Synthesis.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Illuminating the Interface: In Situ Optical Insights Into Two-Electron ORR Pathways for HAdvanced materials (Deerfield Beach, Fla.) · 2026Review
- Preparation of 1,4-Naphthoquinones and 9,10-Anthraquinones through Brønsted Acid-Catalyzed [4+2] Cycloaddition.Organic letters · 2026Article
- Materials Design and Assessment of Redox-Mediated Flow Cell Systems for Enhanced Energy Storage and Conversion.Advanced materials (Deerfield Beach, Fla.) · 2025Article
Corrections and comments
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Authors and funding
6 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Hydrogen peroxide is manufactured industrially via the anthraquinone autoxidation process-a typical thermocatalytic non-aqueous method. Despite a high interest in using renewable electricity to drive such processes, electrifying non-aqueous syntheses remains a substantial challenge. Here we present a multi-phase electrochemical anthraquinone autoxidation process that leverages an aqueous-non-aqueous interfacial proton-coupled electron transfer method facilitated by heterogeneous molecular mediation. This design enables the reduction of aqueous anthraquinones with high efficiency at high current densities, using only carbon electrodes. The method operates with high selectivity through a quinhydrone intermediate and prevents the over-reduction of aromatics during thermocatalytic hydrogenation. This approach combines the benefits of aqueous electrochemistry with those of the traditional non-aqueous process to achieve high current density electrochemistry with rapid kinetics and mass transport, while avoiding unwanted electrolyte in the hydrogen peroxide product. This strategy bridges aqueous electrochemistry with non-aqueous chemistry and establishes a framework for the electrification and decentralization of other non-aqueous chemical processes.
Identifiers
40983725What OpenQuestion holds
Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.