ArticleInternational journal of molecular sciences2025
Activation of Specific Reagents in Molecular Films by Sub-Ionization Electrons: Chlorobenzene/Water Films.
Article in International journal of molecular sciences, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Control over chemical reactivity remains a fundamental challenge in synthesis chemistry, where targeting a specific reactant represents the ultimate goal. While photoactivation is a well-established approach for selective excitation, electron-induced chemistry offers a complementary pathway with high efficacy. In this study, we investigate the effects of low-energy electron irradiation on prototypical chlorobenzene/water molecular films, demonstrating that chlorobenzene can be selectively dissociated via a resonant process occurring at ~1 eV. At higher electron energies (>6 eV), multiple reaction pathways become accessible, including the fragmentation of both water and chlorobenzene molecules. Our study provides a perspective strategy for achieving reagent-specific control in complex molecular assemblies via low-energy electrons, offering new insights into electron-driven surface chemistry and reaction dynamics at the molecular level.
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