Evidence map›Paper›PMID 40942281›Full record

ArticlePolymers2025

Comparative Life Cycle Assessment for the Fabrication of Polysulfone Membranes Using Slot Die Coating as a Scalable Fabrication Technique.

David Lu, Isaac Oluk, Minwoo Jung, Sophia Tseng, Diana M Byrne, Tequila A L Harris, Isabel C Escobar

Abstract read
In one paragraph

Article in Polymers, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.

0numbers the graph read from it
0cells of the map it votes in
3citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

3 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

7 authors.

David LuDepartment of Chemical and Materials Engineering, University of Kentucky, Lexington, KY 40506, USA.ORCID 0000-0002-1973-3197
Isaac OlukDepartment of Civil Engineering, University of Kentucky, Lexington, KY 40506, USA.ORCID 0000-0002-4526-8233
Minwoo JungGeorge W. Woodruff School of Mechanical Engineering, Georgia Institute of Technology, Atlanta, GA 30332, USA.
Sophia TsengDepartment of Chemical and Materials Engineering, University of Kentucky, Lexington, KY 40506, USA.
Diana M ByrneDepartment of Civil Engineering, University of Kentucky, Lexington, KY 40506, USA.ORCID 0000-0002-5793-6024
Tequila A L HarrisGeorge W. Woodruff School of Mechanical Engineering, Georgia Institute of Technology, Atlanta, GA 30332, USA.ORCID 0000-0002-6086-6987
Isabel C EscobarDepartment of Chemical and Materials Engineering, University of Kentucky, Lexington, KY 40506, USA.ORCID 0000-0001-9269-5927

Funding

U.S. National Science Foundation 1922694U.S. National Science Foundation 2121674
6 · The paper itself

Abstract

Despite the emergence of eco-friendly solvents and scalable methods for polymeric membrane fabrication, studies on the impacts of solvent synthesis and manufacturing scale-up have not been conducted. To this end, a life cycle assessment (LCA) was developed with the goal of determining the global environmental and health impacts of producing polysulfone (PSf) membranes with the solvents PolarClean and γ-valerolactone (GVL) via doctor blade extrusion (DBE) and slot die coating (SDC). Along with PolarClean and GVL, dimethylacetamide (DMAc) and N-methyl-2-pyyrolidone (NMP) were included in the LCA as conventional solvents for comparison. The dope solution viscosity had a major influence on the material inventories; to produce a normalized membrane unit on a surface area basis, a larger quantity of PSf-PolarClean-GVL materials was required due to its high viscosity. The life cycle impact assessment found electricity and PolarClean to be major contributing parameters to multiple impact categories during membrane fabrication. The commercial synthesis route of PolarClean selected in this study required hazardous materials derived from petrochemicals, which increased its impact on membrane fabrication. Due to more materials being required to fabricate membranes via SDC to account for tool fluid priming, the PSf-PolarClean-GVL membrane fabricated via SDC exhibited the highest impacts. The amount of electricity and concentration of PolarClean were the most sensitive parameters according to Spearman's rank coefficient analysis. A scenario analysis in which the regional energy grid was substituted found that using the Swedish grid, which comprises far more renewable technologies than the global and US energy grids, significantly lowered impacts in most categories. Despite the reported eco-friendly benefits of using PolarClean and GVL as alternatives to conventional organic solvents, the results in this study provide a wider perspective of membrane fabrication process impacts, highlighting that upstream impacts can counterbalance the beneficial properties of alternative materials.

Indexed as

eco-friendly solventslife cycle assessmentmembranesroll-to-rollsustainability

Identifiers

PMID40942281
PMCPMC12431056

What OpenQuestion holds

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LicenceCC BY
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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.