ArticleMikrochimica acta2025
Enhanced electrochemiluminescence aptasensor using ZnO as the co-reaction accelerator of Mn-NHCDs/TEA system for the detection of florfenicol.
Article in Mikrochimica acta, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
A novel ternary electrochemiluminescence (ECL) aptasensor was creatively proposed for florfenicol (FF) detection, on account of the manganese-nitrogen dual-doped carbon dots (Mn-NHCDs) emitter and the facilitation of triethylamine (TEA) by zinc oxide (ZnO). First, Mn-NHCDs with low excitation potentials and excellent electrochemical luminescence properties were synthesized. Then, a newly formulated ZnO with an enlarged specific surface area and an appropriate mesoporous structure was utilized to load Mn-NHCDs, thereby diminishing the leakage of Mn-NHCDs and stabilizing the luminescence within the system. More importantly, ZnO can serve as a new co-reaction accelerator for TEA to improve the reaction rate of Mn-NHCDs with TEA efficiently. Furthermore, owing to the overlap of spectra, we employed an ECL resonance energy transfer (ECL-RET) strategy, with the Mn-NHCDs/ZnO as the donor and black hole quencher (BHQ) as the acceptor. The ECL biosensor illustrates an extremely selective and sensitive determination of FF from 1.00 fg mL⁻
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