ArticleChemical science2025
Hierarchical hollow nanospheres of imine-based covalent organic frameworks with built-in Ag sites for fast-charging lithium metal batteries.
Article in Chemical science, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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Who cites it
1 citing paper in PubMed.
- Dynamic Ion-Adsorption Interface for Uniform Lithium-Ion Transport in High-Performance Lithium Metal Batteries.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
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Authors and funding
8 authors.
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No grant is acknowledged in the PubMed record.
Abstract
Lithium metal is deemed to be the ultimate anode material for high-energy-density and fast-charging lithium batteries. However, issues of dendritic deposition and frangible solid electrolyte interphases must be resolved for lithium metal anodes. Herein, a hybrid interfacial layer, hierarchical hollow nanospheres assembled from lithiophilic imine-based covalent organic frameworks and built-in Ag sites (Ag@ICOFs), has been applied to regulate the interfacial lithium ion flux and enhance the anode stability for effectively inhibiting dendrite formation. The hollow ICOFs play important roles in enhancing electrolyte infiltration caused by ordered porous channels and promoting uniform lithium distribution due to the superior lithiophilic ability of binding sites (C[double bond, length as m-dash]N groups and benzene rings). Moreover, the filling of Ag can induce internal deposition in hollow Ag@ICOFs nanospheres when lithium metal tends to grow vertically. The dendrite-free lithium development is further verified by
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