ArticleBiomacromolecules2025
Sustainable Hybrid Latexes Derived from Starch Bioparticles and Biobased Monomers.
Article in Biomacromolecules, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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7 authors.
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Abstract
Starch is a widely available biopolymer with the potential to replace petroleum-based acrylic monomers in coating binders, but its hydrophilicity and water sensitivity limit its incorporation. This study enhances biobased content in hybrid latexes by simultaneously incorporating starch/zein bioparticles (BPs), produced via nanoprecipitation, and commercial biobased monomers including 2-octyl acrylate, 2-octyl methacrylate, and isobornyl methacrylate. Waterborne hybrid dispersions were synthesized through semibatch emulsion polymerization, using BPs as seeds with variable biobased formulations. The influence of solids content, increased from 20% to 32%, was also examined. The resulting hybrid latexes achieved biobased contents exceeding 70% and demonstrated excellent film-forming properties. When applied in paint formulations, they yielded stable coatings with high surface hydrophobicity (contact angle of 98°) and good coverage. These findings demonstrate the potential of combining starch-based bioparticles with bioderived monomers to create sustainable waterborne coatings with high biobased content and competitive performance.
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