ArticleNature communications2025
Dynamic construction of a durable epitaxial catalytic layer for industrial alkaline water splitting.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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Who cites it
4 citing papers in PubMed.
- Lattice strain engineering of iridium-based catalysts for acidic oxygen evolution reaction.Chemical science · 2026Review
- Regulating the Electronic Structure via Multi-Transition Metals in Nanoporous High-Entropy Perovskites for Boosted Alkaline Hydrogen Evolution.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Energy-efficient bifunctional CoBRSC advances · 2025Article
- Hierarchical Porous P-Doped NiCo Alloy with α/ε Phase-Defect Synergy to Boost Alkaline HER Kinetics and Bifunctional Activity.Nanomaterials (Basel, Switzerland) · 2025Article
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Authors and funding
18 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Optimizing the catalyst-electrolyte interface structure is crucial for enhancing the performance of electrochemical alkaline hydrogen evolution reaction. Traditional approaches typically focus on regulating the thermodynamic barriers of adsorption and desorption for reactants, intermediates, and ions at active sites on the solid electrode surface. However, the structure of the electrical double layer influences the concentration of intermediates, adsorption energy, and surface reaction kinetics. Here, we dynamically construct a dense epitaxial hydroxide layer on nickel molybdate, forming an effective protective barrier to prevent molybdenum leaching and enhance material stability. This optimization enhances local electric field increasing the concentration of hydrated potassium ions within the outer Helmholtz plane. As a result, the interfacial hydrogen-bond network improves, water availability on the catalyst surface increases, and reaction kinetics accelerate. The optimized material operates stably for 1400 h at a current density of 0.45 A cm
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Registered trials
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