Evidence map›Paper›PMID 40856038›Full record

ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2025

Regulating Spin Polarization through Topological Defects in Carbon-Based Metal-Free Catalyst for Enhanced Fenton-Like Activity.

Huajie Zhong, Zeyu Gong, Xi Chen, Bin Zhang, Tao Zhan, Jiaxing Yu, Yu Hou, Yuan Tao, Qi Fu, Huangsheng Yang and 5 more

Abstract read
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In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

0numbers the graph read from it
0cells of the map it votes in
1citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

1 citing paper in PubMed.

  1. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

15 authors.

Huajie ZhongSchool of Chemical Engineering and Technology, Sun Yat-Sen University, Zhuhai, Guangdong, 519082, P. R. China.
Zeyu GongSchool of Chemical Engineering and Technology, Sun Yat-Sen University, Zhuhai, Guangdong, 519082, P. R. China.
Xi ChenSchool of Chemical Engineering and Technology, Sun Yat-Sen University, Zhuhai, Guangdong, 519082, P. R. China.
Bin ZhangSchool of Biology and Biological Engineering, South China University of Technology, Guangzhou, Guangdong, 510006, P. R. China.
Tao ZhanSchool of Chemical Engineering and Technology, Sun Yat-Sen University, Zhuhai, Guangdong, 519082, P. R. China.
Jiaxing YuMOE Key Laboratory of Bioinorganic and Synthetic Chemistry/KLGHEI of Environment and Energy Chemistry, School of Chemistry, Sun Yat-Sen University, Guangzhou, Guangdong, 510275, P. R. China.
Yu HouGuangzhou Customs Technology Center, Guangzhou, Guangdong, 510623, P. R. China.
Yuan TaoSchool of Biology and Biological Engineering, South China University of Technology, Guangzhou, Guangdong, 510006, P. R. China.
Qi FuSchool of Biology and Biological Engineering, South China University of Technology, Guangzhou, Guangdong, 510006, P. R. China.
Huangsheng YangSchool of Biology and Biological Engineering, South China University of Technology, Guangzhou, Guangdong, 510006, P. R. China.
Jiating ZhengSchool of Chemical Engineering and Technology, Sun Yat-Sen University, Zhuhai, Guangdong, 519082, P. R. China.
Duochu SuFoshan Fosun Chancheng Hospital, Foshan, Guangdong, 528000, P. R. China.
Ganggang LiNational Engineering Laboratory for VOCs pollution Control Material & Technology, Research Center for Environmental Material and Pollution Control Technology, University of Chinese Academy of Sciences, Beijing, 101408, P.R. China.
Junhui WangSchool of Chemical Engineering and Technology, Sun Yat-Sen University, Zhuhai, Guangdong, 519082, P. R. China.
Gangfeng OuyangSchool of Chemical Engineering and Technology, Sun Yat-Sen University, Zhuhai, Guangdong, 519082, P. R. China.ORCID https://orcid.org/0000-0002-0797-6036

Funding

Fundamental Research Funds for the Central Universities SunYat-senUniversity[24lgqb013]Guangdong Basic Research Center of Excellence for Functional Molecular EngineeringGuangdong Provincial Key R&D Programme 2020B1111350002Guangzhou Science and Technology Planning Project 202206010074National Natural Science Foundation Projects 22036003National Natural Science Foundation Projects 22076222Natural Science Foundation of Guangdong Province 2024A1515030070Science and Technology Program of Guangzhou Project 202102021203
6 · The paper itself

Abstract

Regulating spin polarization has been recognized as a promising strategy to improve the catalytic performance across various catalytic domains, since the reaction barriers can be directly influenced by the spin state. However, the existing approaches to modulating the spin polarization of active centers mainly focus on the metal-based catalysts, and those for the earth-abundant carbon-based metal-free catalysts (CMFCs) are rarely reported. Here, a topological defect engineering strategy is proposed to regulate the spin polarization by introducing pentagon defects on the edge of CMFCs. Theoretical and experimental results indicate that the incorporation of pentagon defects on the edge induces a spin polarization, and more spin-down electrons locate below the Fermi level, which enhances the electron transfer between peroxymonosulfate (PMS) and the catalyst, and reduces the energy barrier of the key

Indexed as

carbocatalystscarbon defectFenton‐like reactionspin polarization

Identifiers

PMID40856038
PMCPMC12622554

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.