Ultrahigh-Temperature-Tolerance Lithium Metal Batteries Enabled by Molecular-Level Polymer Configuration Design with Low-Entropy-Penalty Effect.

Weiting Ma, Shunshun Zhao, Shuang Wan, Jiajun Gong, Sinian Yang, Yong Chen, Shimou Chen, Guoxiu Wang

Abstract read

In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it

0cells of the map it votes in

2citing papers in PubMed

–field-weighted citation impact

1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

Deep Eutectic Electrolytes for Lithium Metal Batteries: A Review.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026
Review
Ultrahigh-Temperature-Tolerance Lithium Metal Batteries Enabled by Molecular-Level Polymer Configuration Design with Low-Entropy-Penalty Effect.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025
Article

4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

8 authors.

Weiting MaState Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology of Materials, Beijing University of Chemical Technology, Beijing, 100029, P. R. China.

Shunshun ZhaoState Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology of Materials, Beijing University of Chemical Technology, Beijing, 100029, P. R. China.

Shuang WanState Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology of Materials, Beijing University of Chemical Technology, Beijing, 100029, P. R. China.

Jiajun GongState Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology of Materials, Beijing University of Chemical Technology, Beijing, 100029, P. R. China.

Sinian YangState Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology of Materials, Beijing University of Chemical Technology, Beijing, 100029, P. R. China.

Yong ChenCentre for Clean Energy Technology, University of Technology Sydney, Broadway, Sydney, NSW, 2007, Australia.ORCID https://orcid.org/0000-0003-1515-7708

Shimou ChenState Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology of Materials, Beijing University of Chemical Technology, Beijing, 100029, P. R. China.

Guoxiu WangCentre for Clean Energy Technology, University of Technology Sydney, Broadway, Sydney, NSW, 2007, Australia.ORCID https://orcid.org/0000-0003-4295-8578

Funding

ARC Linkage project LP200200926Australian Research Council DP240102176Beijing Natural Science Foundation L245007Fundamental Research Funds for the Central Universities buctrc202104National Natural Science Foundation of China 52171198National Natural Science Foundation of China 52425207

6 · The paper itself

Abstract

Despite their immense potential for next-generation energy storage, the practical implementation of temperature-tolerant lithium metal batteries (LMBs) under extreme thermal conditions continues to face formidable challenges. In this study, an ultrahigh-temperature-tolerance polymer-based electrolyte (UPE) prototype with a low-entropy-penalty effect is proposed. This electrolyte features a carefully engineered molecular configuration that enables stable operation of polymer-based LMBs across a broad temperature range (25-150 °C). Comprehensive experimental and theoretical analyses confirm that the unique "ester-ether-fluorinated segment" architecture enables the formation of a robust coordination framework through Li⁺-multivalent ether/ester interactions and effective Li

Indexed as

lithium metal batterieslow‐entropy penaltypolymer electrolyteultrahigh‐temperature‐tolerance

Identifiers

PMID40817755

DOI10.1002/advs.202507191

PMCPMC12591149

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.