ArticleThe journal of physical chemistry letters2025
Impact of Dark Polariton States on Collective Strong Light-Matter Coupling in Molecules.
Article in The journal of physical chemistry letters, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Cavity-modified exciton-exciton annihilation in disordered molecular systems.Physical chemistry chemical physics : PCCP · 2026Article
- A macroscopic condensation theory for vibrational strong coupling effects.Nature communications · 2026Article
- Quantum Dynamics Simulations of Polariton Transport in a Bloch Surface Wave Cavity.Nanophotonics (Berlin, Germany) · 2026Article
- Polariton Control of Molecular Charge Transfer in Perylene Diimide Semiconductors.The journal of physical chemistry letters · 2026Article
- Collectively-Modified Intermolecular Electron Correlations: The Connection of Polaritonic Chemistry and Spin Glass Physics.Chemical reviews · 2026Review
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Authors and funding
3 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Polaritonic chemistry investigates the possible modification of chemical and photochemical reactions by means of strong light-matter coupling in optical cavities, as demonstrated in numerous experiments over the past few years. These experiments are typically interpreted in terms of the Jaynes-Cummings or Tavis-Cummings models under the assumption that the molecular ensemble is only excited by a single photon. In such a model, two polariton states compete with an overwhelming number of dark states, inhibiting polaritonic reactions entropically. We analyze the higher excitation manifolds of the Tavis-Cummings model along with a three-level system that resembles photochemical reactions. We demonstrate that allowing for more than a single excitation makes the reaction of the involved polaritons entropically more favorable.
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Registered trials
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